Abstract
Fundamental research on two-dimensional (2D) magnetic systems based on van der Waals materials has been rapidly gaining traction since their recent discovery. With the increase of recent knowledge, it has become clear that such materials have also a strong potential for applications in devices that combine magnetism with electronics, optics, and nanomechanics. Nonetheless, many challenges still lay ahead. Several fundamental aspects of 2D magnetic materials are still unknown or poorly understood, such as their often-complicated electronic structure, optical properties, magnetization dynamics, and magnon spectrum. To elucidate their properties and facilitate integration in devices, advanced characterization techniques and theoretical frameworks need to be developed or adapted. Moreover, developing synthesis methods which increase critical temperatures and achieve large-scale, high-quality homogeneous thin films is crucial before these materials can be used for real-world applications. Therefore, the field of 2D magnetic materials provides many challenges and opportunities for the discovery and exploration of new phenomena, as well as the development of new applications. This Roadmap presents the background, challenges, and potential research directions across key topics in the field, including fundamentals, synthesis, characterization, and applications. We hope that this work can provide a strong starting point for young researchers in the field and provide a general overview of the key challenges for more experienced researchers.
| Original language | English |
|---|---|
| Article number | 031501 |
| Number of pages | 55 |
| Journal | 2D Materials |
| Volume | 12 |
| Issue number | 3 |
| Early online date | 10 Mar 2025 |
| DOIs | |
| Publication status | Published - Jul 2025 |
Bibliographical note
Publisher Copyright:© 2025 The Author(s). Published by IOP Publishing Ltd.
Funding
We are thankful to the Lorentz Centre in Leiden, the Netherlands, for hosting the workshop on Quantum Magnetic Materials (Oct. 2023), which provided the opportunity to carry the initial discussions which lead to the writing of this article. AGC, ZZ and MHDG acknowledge the research program “Materials for the Quantum Age” (QuMat) for financial support. This program (registration number 024.005.006) is part of the Gravitation program financed by the Dutch Ministry of Education, Culture and Science (OCW). MHDG acknowledges the financial support of the European Union through grant ERC, 2D-OPTOSPIN, 101076932, the Dutch Research Council (NWO—OCENW.XL21.XL21.058). MHDG and AGC acknowledge the financial support of the Zernike Institute for Advanced Materials. ZZ has received funding from the European Union’s Horizon Europe research and innovation programme under grant agreement No 101130384 (QUONDENSATE). DS acknowledges financial support from Generalitat Valenciana through the CIDEGENT program (CIDEGENT/2021/052) and the Advanced Materials program by MCIN with funding from European Union NextGenerationEU (MFA/2022/045). AGC acknowlegdes help from Dr. Falk Pabst in the preparation of the table of materials
| Funder number | |
|---|---|
| ???publication-publication-funding-organisation-not-added??? | 024.005.006 |
| ???publication-publication-funding-organisation-not-added??? | 101130384 |
Keywords
- 2D magnets
- applications
- moiré magnets
- spintronics
- strong correlations
- synthesis and fabrication
- van der Waals heterostructures
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