Photothermal heterodyne imaging of individual metallic nanoparticles: Theory versus experiment

Stéphane Berciaud*, David Lasne, Gerhard A. Blab, Laurent Cognet, Brahim Lounis

*Corresponding author for this work

Research output: Contribution to journalArticleAcademicpeer-review

Abstract

We present the theoretical and detailed experimental characterizations of photothermal heterodyne imaging. An analytical expression of the photothermal heterodyne signal is derived using the theory of light scattering from a fluctuating medium. The amplitudes of the signals detected in the backward and forward configurations are compared and their frequency dependences are studied. The application of the photothermal heterodyne detection technique to the absorption spectroscopy of individual gold nanoparticles is discussed and the detection of small individual silver nanoparticles is demonstrated.

Original languageEnglish
Article number045424
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume73
Issue number4
DOIs
Publication statusPublished - 2006

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