Abstract
Detailed spatial models of monthly air pollution levels at a very fine spatial resolution (25 m) can help facilitate studies to explore critical time-windows of exposure at intermediate term. Seasonal changes in air pollution may affect both levels and spatial patterns of air pollution across Europe. We built Europe-wide land-use regression (LUR) models to estimate monthly concentrations of regulated air pollutants (NO2, O3, PM10 and PM2.5) between 2000 and 2019. Monthly average concentrations were collected from routine monitoring stations. Including both monthly-fixed and -varying spatial variables, we used supervised linear regression (SLR) to select predictors and geographically weighted regression (GWR) to estimate spatially-varying regression coefficients for each month. Model performance was assessed with 5-fold cross-validation (CV). We also compared the performance of the monthly LUR models with monthly adjusted concentrations. Results revealed significant monthly variations in both estimates and model structure, particularly for O3, PM10, and PM2.5. The 5-fold CV showed generally good performance of the monthly GWR models across months and years (5-fold CV R2: 0.31–0.66 for NO2, 0.4–0.79 for O3, 0.4–0.78 for PM10, 0.46–0.87 for PM2.5). Monthly GWR models slightly outperformed monthly-adjusted models. Correlations between monthly GWR model were generally moderate to high (Pearson correlation >0.6). In conclusion, we are the first to develop robust monthly LUR models for air pollution in Europe. These monthly LUR models, at a 25 m spatial resolution, enhance epidemiologists to better characterize Europe-wide intermediate-term health effects related to air pollution, facilitating investigations into critical exposure time windows in birth cohort studies.
| Original language | English |
|---|---|
| Article number | 170550 |
| Pages (from-to) | 1-16 |
| Number of pages | 16 |
| Journal | Science of the Total Environment |
| Volume | 918 |
| Early online date | 4 Feb 2024 |
| DOIs | |
| Publication status | Published - 25 Mar 2024 |
Bibliographical note
Publisher Copyright:© 2024 The Authors
Funding
This work was supported by EXPANSE and EXPOSOME-NL project. The EXPANSE project is funded by the European Union's Horizon 2020 research and innovation programme under grant agreement No 874627. The content of this article is not officially endorsed by the European Union. The EXPOSOME-NL project is funded through the Gravitation program of the Dutch Ministry of Education, Culture, and Science and the Netherlands Organization for Scientific Research (NWO grant number 024.004.017) . The computation was done with SURF Research Cloud infrastructure with grant no. SD -19729. The authors declare no competing financial interest.
| Funders | Funder number |
|---|---|
| Dutch Ministry of Education, Culture, and Science | |
| EXPANSE | |
| EXPOSOME-NL | |
| European Commission | |
| Nederlandse Organisatie voor Wetenschappelijk Onderzoek | SD-19729, 024.004.017 |
| Horizon 2020 | 874627 |
UN SDGs
This output contributes to the following UN Sustainable Development Goals (SDGs)
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SDG 15 Life on Land
Keywords
- Air pollution
- Europe-wide
- Land-use regression
- Monthly variation
- Spatiotemporal variation
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