FUEL 228-Methoxy functionalized palladium triphenylphosphine complexes: Active catalysts for the telomerization of crude glycerol

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Abstract

Potential applications for the increasing amount of glycerol as by-product in the biodiesel production are of growing interest. A promising reaction type is the telomerization of glycerol with 1,3-butadiene leading to C8-chain ethers of glycerol applicable in polymer and surfactant chemistry or as chemical building blocks. In this study, we present a new catalyst system for the telomerization of glycerol with butadiene applying palladium-based triphenylphosphine complexes with methoxy functionalized ring systems. The resulting complexes show remarkable activity under various reaction conditions. Particularly, the catalyst system is capable to directly convert crude glycerol without any significant loss of activity, thus providing an interesting route from cheap starting materials towards high added value products.

Original languageEnglish
Number of pages1
JournalACS National Meeting Book of Abstracts
Volume235
Publication statusPublished - 6 Apr 2008
Event235th National Meeting of the American Chemical Society, ACS 2008 - New Orleans, LA, United States
Duration: 6 Apr 200810 Apr 2008

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