Abstract
Previous European land-use regression (LUR) models assumed fixed linear relationships between air pollution concentrations and predictors such as traffic and land use. We evaluated whether including spatially-varying relationships could improve European LUR models by using geographically weighted regression (GWR) and random forest (RF). We built separate LUR models for each year from 2000 to 2019 for NO2, O3, PM2.5 and PM10 using annual average monitoring observations across Europe. Potential predictors included satellite retrievals, chemical transport model estimates and land-use variables. Supervised linear regression (SLR) was used to select predictors, and then GWR estimated the potentially spatially-varying coefficients. We developed multi-year models using geographically and temporally weighted regression (GTWR). Five-fold cross-validation per year showed that GWR and GTWR explained similar spatial variations in annual average concentrations (average R2 = NO2: 0.66; O3: 0.58; PM10: 0.62; PM2.5: 0.77), which are better than SLR (average R2 = NO2: 0.61; O3: 0.46; PM10: 0.51; PM2.5: 0.75) and RF (average R2 = NO2: 0.64; O3: 0.53; PM10: 0.56; PM2.5: 0.67). The GTWR predictions and a previously-used method of back-extrapolating 2010 model predictions using CTM were overall highly correlated (R2 > 0.8) for all pollutants. Including spatially-varying relationships using GWR modestly improved European air pollution annual LUR models, allowing time-varying exposure-health risk models.
Original language | English |
---|---|
Article number | 107485 |
Pages (from-to) | 1-12 |
Number of pages | 12 |
Journal | Environment international |
Volume | 168 |
DOIs | |
Publication status | Published - Oct 2022 |
Bibliographical note
Funding Information:This work was supported by EXPANSE and EXPOSOME-NL projects. The EXPANSE project is funded by the European Union’s Horizon 2020 research and innovation programme under grant agreement No 874627. The content of this article is not officially endorsed by the European Union. The EXPOSOME-NL project is funded through the Gravitation programme of the Dutch Ministry of Education, Culture, and Science and the Netherlands Organization for Scientific Research (NWO grant number 024.004.017). The authors declare no competing financial interest.
Funding Information:
This work was supported by EXPANSE and EXPOSOME-NL projects. The EXPANSE project is funded by the European Union's Horizon 2020 research and innovation programme under grant agreement No 874627. The content of this article is not officially endorsed by the European Union. The EXPOSOME-NL project is funded through the Gravitation programme of the Dutch Ministry of Education, Culture, and Science and the Netherlands Organization for Scientific Research (NWO grant number 024.004.017). The authors declare no competing financial interest.
Publisher Copyright:
© 2022 The Author(s)
Funding
This work was supported by EXPANSE and EXPOSOME-NL projects. The EXPANSE project is funded by the European Union’s Horizon 2020 research and innovation programme under grant agreement No 874627. The content of this article is not officially endorsed by the European Union. The EXPOSOME-NL project is funded through the Gravitation programme of the Dutch Ministry of Education, Culture, and Science and the Netherlands Organization for Scientific Research (NWO grant number 024.004.017). The authors declare no competing financial interest. This work was supported by EXPANSE and EXPOSOME-NL projects. The EXPANSE project is funded by the European Union's Horizon 2020 research and innovation programme under grant agreement No 874627. The content of this article is not officially endorsed by the European Union. The EXPOSOME-NL project is funded through the Gravitation programme of the Dutch Ministry of Education, Culture, and Science and the Netherlands Organization for Scientific Research (NWO grant number 024.004.017). The authors declare no competing financial interest.
Keywords
- Geographically and temporally weighted regression
- Land-use regression
- Random forest
- Spatially varying coefficient
- Spatiotemporal variation