Enantioselective dialkylation of 1,2-phthalicdicarboxaldehyde

Henk Kleijn, Johann T.B.H. Jastrzebski, Jaap Boersma, Gerard Van Koten

Research output: Contribution to journalArticleAcademicpeer-review

Abstract

A new two-step, one-pot procedure is reported for the enantioselective synthesis of C2-symmetric diols derived from 1,2-phthalicdicarboxaldehyde. The first step involves the enantioselective addition of a dialkylzinc compound to one of the aldehyde groups, affording a lactol organozinc derivative. In the second step this lactol derivative is converted to the appropriate diol with the aid of a Grignard reagent and subsequent hydrolysis. This methodology also allows the synthesis of unsymmetric diols. © 2001 Elsevier Science Ltd.
Original languageEnglish
Pages (from-to)3933-3937
Number of pages5
JournalTetrahedron Letters
Volume42
Issue number23
DOIs
Publication statusPublished - 4 Jun 2001

Keywords

  • 1,2 phthalicarboxaldehyde
  • aldehyde derivative
  • Grignard reagent
  • lactone derivative
  • reagent
  • unclassified drug
  • alkylation
  • article
  • chemical reaction
  • diastereoisomer
  • enantiomer
  • hydrolysis
  • stereochemistry
  • synthesis

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