Abstract
sn-1-Diacylglycerol lipase α (DAGL-α) is the main enzyme responsible for the production of the endocannabinoid 2-arachidonoylglycerol in the central nervous system. Glycine sulfonamides have recently been identified by a high throughput screening campaign as a novel class of inhibitors for this enzyme. Here, we report on the first structure-activity relationship study of glycine sulfonamide inhibitors and their brain membrane proteome-wide selectivity on serine hydrolases with activity-based protein profiling (ABPP). We found that (i) DAGL-α tolerates a variety of biaryl substituents, (ii) the sulfonamide is required for inducing a specific orientation of the 2,2-dimethylchroman substituent, and (iii) a carboxylic acid is essential for its activity. ABPP revealed that the sulfonamide glycine inhibitors have at least three off-targets, including α/β-hydrolase domain 6 (ABHD6). Finally, we identified LEI-106 as a potent, dual DAGL-α/ABHD6 inhibitor, which makes this compound a potential lead for the discovery of new molecular therapies for diet-induced obesity and metabolic syndrome.
Original language | English |
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Pages (from-to) | 6610-6622 |
Number of pages | 13 |
Journal | Journal of Medicinal Chemistry |
Volume | 57 |
Issue number | 15 |
DOIs | |
Publication status | Published - 14 Aug 2014 |
Externally published | Yes |
Keywords
- Animals
- Brain/metabolism
- Glycine/analogs & derivatives
- HEK293 Cells
- Humans
- Lipoprotein Lipase/antagonists & inhibitors
- Mice
- Models, Molecular
- Monoacylglycerol Lipases/antagonists & inhibitors
- Proteome/metabolism
- Structure-Activity Relationship
- Sulfonamides/chemistry