Autonomously Probing Viscoelasticity in Disordered Suspensions

Clara Abaurrea-Velasco*, Celia Lozano, Clemens Bechinger, Joost De Graaf

*Corresponding author for this work

Research output: Contribution to journalArticleAcademicpeer-review

Abstract

Recent experiments show a strong rotational diffusion enhancement for self-propelled microrheological probes in colloidal glasses. Here, we provide microscopic understanding using simulations with a frictional probe-medium coupling that converts active translation into rotation. Diffusive enhancement emerges from the medium's disordered structure and peaks at a second-order transition in the number of contacts. Our results reproduce the salient features of the colloidal glass experiment and support an effective description that is applicable to a broader class of viscoelastic suspensions.

Original languageEnglish
Article number258002
JournalPhysical Review Letters
Volume125
Issue number25
DOIs
Publication statusPublished - 18 Dec 2020

Funding

J. d G. gratefully recognizes the Dutch Research Council (NWO) for funding this research through Start-Up Grant No. 740.018.013. C. B. acknowledges financial support by the ERC Advanced Grant ASCIR (Grant No. 693683) and by the German Research Foundation (DFG) through the priority programme SPP 1726. We thank F. Smallenburg, M. Hermes, and L. Filion for useful discussions. Conceptualization, J. d G.; methodology, C. A. V., C. L., C. B., and J. d G.; software, C. A. V.; validation, C. A. V. (lead) and C. L. and J. d G. (supporting); investigation, C. A. V. (lead) and C. L. (supporting); original draft, C. A. V. and J. d G.; review and editing, J. d G., C. B., C. A. V., and C. L.; funding acquisition, resources, and supervision, J. d G. and C. B.

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