A comparative energy and costs assessment and optimization for direct air capture technologies

Francesco Sabatino, Alexa Grimm, Fausto Gallucci, Martin van Sint Annaland, Gert Jan Kramer, Matteo Gazzani*

*Corresponding author for this work

Research output: Contribution to journalArticleAcademicpeer-review

Abstract

This work provides a comparative technical assessment of three technologies for CO2 removal from air: two aqueous-scrubbing processes and one solid sorbent process. We compute productivity and exergy and energy consumption using process simulations and mathematical optimization. Moreover, we evaluate the cost range and discuss the challenges for large-scale deployment. We show that all technologies can provide high-purity CO2 and that the solid-based process has the potential to offer the best performance, owing to an exergy demand of 1.4–3.7 MJ.kgCO2−1 and a productivity of 3.8–10.6 kgCO2.m−3.h−1. Translating productivity and energy into cost of CO2 capture via a simple model, we show that the capital cost is the main cost driver. All technologies have the potential to operate below 200 $.tonCO2−1 under favorable, yet realistic, energy and reactor costs. The solid-sorbent process achieves this under a broader range of conditions and is less dependent on the installation cost when a high mass transfer is achieved.

Original languageEnglish
Pages (from-to)2047-2076
Number of pages30
JournalJoule
Volume5
Issue number8
DOIs
Publication statusPublished - 18 Aug 2021

Keywords

  • CCS
  • CDR
  • DAC
  • direct air capture
  • negative emissions technologies
  • net zero emissions
  • optimization
  • process modelling
  • solid sorbents
  • tecno-economic assessment

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